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Variational quantum eigensolver

The variational quantum eigensolver (VQE) is a hybrid quantum-classical designed to approximate the ground-state and wavefunction of a quantum system by variationally minimizing the expectation value of its using a parameterized prepared on a quantum , combined with classical optimization techniques. Introduced in on a photonic quantum , VQE leverages the from , which guarantees that the computed provides an upper bound to the true ground-state , making it particularly suitable for noisy intermediate-scale quantum (NISQ) devices with limited coherence times compared to methods like quantum phase estimation. Key components of VQE include the , a parameterized that generates trial wavefunctions (often inspired by classical methods like unitary coupled cluster for chemistry applications); the measurement strategy, which computes the expectation value of the Hamiltonian's Pauli terms on the quantum hardware; and the classical optimizer, such as or derivative-free methods like COBYLA, which iteratively adjusts the ansatz parameters to minimize the energy. This iterative process allows VQE to handle complex many-body Hamiltonians that are intractable on classical computers, with demonstrated applications in for molecules like H₂ and He–H⁺, as well as in for modeling Ising models and frustrated magnets. Since its inception, VQE has evolved with advancements in error mitigation techniques, such as zero-noise extrapolation and readout error correction, to improve accuracy on current hardware, and extensions like adaptive ansatzes that dynamically build circuits to reduce circuit depth and barren plateaus in the optimization landscape. Ongoing research addresses challenges including measurement overhead, noise resilience, and , positioning VQE as a for near-term quantum simulations in fields ranging from to materials design, though quantum advantage remains contingent on mitigating large prefactors in computational cost.

Introduction

Overview

The Variational Quantum Eigensolver (VQE) is a quantum-classical designed to approximate the ground-state and corresponding wavefunction of a quantum system by preparing variational trial states using parameterized quantum circuits and minimizing the expectation value of the system's through classical optimization. This approach leverages the , ensuring that the resulting serves as an upper bound to the true ground-state value, while the —representing the total of the system—is encoded into measurable observables on the quantum hardware. VQE has emerged as a key method in the Noisy Intermediate-Scale Quantum (NISQ) era, where quantum devices with 50–100 qubits and imperfect gates limit the feasibility of fully fault-tolerant algorithms. It addresses quantum many-body problems, such as simulating molecular electronic structures for applications, which scale exponentially and become intractable on classical computers for systems beyond a few atoms. By requiring only short-depth circuits and tolerating noise through iterative refinement, VQE enables practical computations on current quantum hardware without the need for error correction. At a high level, the algorithm proceeds by initializing parameters for a quantum circuit on the quantum processor to generate a trial , measuring the expectation value via repeated executions, and feeding these results to a classical routine that adjusts the parameters to lower the until convergence. This iterative hybrid loop exploits the strengths of both quantum preparation and classical optimization, making VQE suitable for exploring states in and beyond.

History

The variational quantum eigensolver (VQE) originated in 2014 with the work of Peruzzo et al., who introduced it as a hybrid quantum-classical algorithm to approximate ground-state energies of molecular Hamiltonians using limited quantum resources. Their approach leveraged the within a photonic quantum processor, enabling practical simulations despite hardware noise. This marked a pivotal shift toward near-term quantum algorithms suitable for noisy intermediate-scale quantum (NISQ) devices. A key early milestone was the first experimental demonstration of VQE on the He–H⁺ molecule in the same 2014 study, where Peruzzo et al. achieved chemical accuracy for bond dissociation energies using a four- setup. In 2016, VQE was extended to the H₂ molecule on superconducting . Subsequent extensions in 2017 by Kandala et al. advanced the method by introducing hardware-efficient ansatze optimized for superconducting quantum processors, alongside readout error mitigation techniques to enhance reliability on multi- systems. Further developments included explorations of unitary coupled-cluster ansatze, which provided chemically inspired trial wavefunctions for improved expressivity, as detailed in the comprehensive review by McArdle et al. From 2018 onward, VQE gained widespread accessibility through integration into open-source frameworks such as IBM's (via its Aqua chemistry module) and Google's Cirq paired with OpenFermion, enabling standardized implementations and simulations across diverse hardware backends. The focus on NISQ-era applications intensified after Google's 2019 Sycamore experiment demonstrated quantum , prompting refinements in VQE toward hardware-efficient ansatze that minimize circuit depth and error accumulation on available processors.

Theoretical Foundations

Variational Principle

The variational theorem, a cornerstone of , states that for a Hermitian operator H with ground-state eigenvector |\psi_0\rangle and corresponding eigenvalue E_0, the expectation value \langle \psi | H | \psi \rangle for any normalized trial state |\psi\rangle satisfies \langle \psi | H | \psi \rangle \geq E_0, with equality holding only if |\psi\rangle = |\psi_0\rangle. This principle, often expressed through the R(\psi) = \frac{\langle \psi | H | \psi \rangle}{\langle \psi | \psi \rangle}, ensures that the ground-state energy minimizes the energy functional over the . The proof relies on the Rayleigh-Ritz method, which approximates the by minimizing the over a finite-dimensional trial manifold spanned by basis functions. Consider a trial state |\phi(\mathbf{a})\rangle = \sum_i a_i |\phi_i\rangle in a subspace of dimension N; the estimated energy is E_{\text{est}}(\mathbf{a}) = \frac{\sum_{i,j} a_i^* a_j \langle \phi_i | H | \phi_j \rangle}{\sum_{i,j} a_i^* a_j \langle \phi_i | \phi_j \rangle}, minimized by solving the generalized eigenvalue problem \det(H - \lambda S) = 0, where H_{ij} = \langle \phi_i | H | \phi_j \rangle and S_{ij} = \langle \phi_i | \phi_j \rangle. The lowest eigenvalue of this matrix provides an upper bound to E_0, as the subspace projection restricts the minimization, and expanding the basis monotonically decreases the estimates toward the exact value from above. In the context of quantum computing, this principle extends to parameterized trial states prepared on quantum hardware, such as variational quantum circuits |\psi(\boldsymbol{\theta})\rangle = U(\boldsymbol{\theta}) |\psi_{\text{init}}\rangle, where U(\boldsymbol{\theta}) is a parameterized and \boldsymbol{\theta} denotes tunable parameters. The Rayleigh quotient is then approximated by measuring \langle \psi(\boldsymbol{\theta}) | H | \psi(\boldsymbol{\theta})\rangle on the device, enabling hybrid quantum-classical optimization to approach the within hardware constraints. A key implication for the variational quantum eigensolver (VQE) is its provision of rigorous upper bounds on the ground-state energy, as the variational theorem guarantees that any computed expectation value exceeds or equals E_0, offering a quantifiable measure of quality without requiring full over the system evolution. This property distinguishes VQE from phase estimation methods and facilitates reliable assessment in noisy intermediate-scale quantum devices.

Quantum Hamiltonians and Encoding

In the context of the variational quantum eigensolver (VQE), quantum Hamiltonians relevant to applications like are typically formulated in second-quantized form to describe fermionic systems, such as electrons in molecules. This representation leverages (\hat{a}^\dagger_p) and annihilation (\hat{a}_q) operators that obey anticommutation relations, efficiently capturing the many-body of the problem while reducing the dimensionality compared to . The general form of the electronic is \hat{H} = \sum_{p,q} h_{pq} \hat{a}^\dagger_p \hat{a}_q + \frac{1}{2} \sum_{p,q,r,s} h_{pqrs} \hat{a}^\dagger_p \hat{a}^\dagger_q \hat{a}_s \hat{a}_r, where the sums run over spin-orbital indices, h_{pq} are one-electron integrals (including and ), and h_{pqrs} are two-electron repulsion integrals, ensuring antisymmetry under particle . This structure arises from the Born-Oppenheimer approximation and Hartree-Fock basis sets, making it central to simulating molecular ground states. To execute VQE on gate-based quantum computers, which operate on s, the fermionic must be mapped to an equivalent operator in the qubit space. This fermion-to-qubit transformation preserves the algebra of the fermionic operators while expressing them as products of (\hat{I}, \hat{X}, \hat{Y}, \hat{Z}). Two seminal mappings are the Jordan-Wigner and Bravyi-Kitaev transformations, both requiring one per spin-orbital for an N-orbital system, thus incurring a linear qubit overhead in the basis set size. The Jordan-Wigner transformation, originally proposed for spin chains but adapted for fermions in simulations, encodes each fermionic mode as a and represents creation operators as \hat{a}^\dagger_j = \frac{1}{2} (\hat{X}_j - i \hat{Y}_j) \prod_{k=0}^{j-1} \hat{Z}_k, with a similar form for annihilation operators; this introduces long-range string operators that enforce the Pauli exclusion principle but result in Pauli terms with weights up to O(N), leading to non-local interactions. In contrast, the Bravyi-Kitaev transformation uses a binary tree (or Fenwick tree) structure to balance occupation number and parity encoding, yielding more local operators with typical Pauli weights of O(\log N); for instance, the creation operator takes the form \hat{a}^\dagger_j = \frac{1}{2} \hat{Z}_{P(j)} \otimes (\hat{X}_j - i \hat{Y}_j) \otimes \prod_{u \in U(j)} \hat{X}_u, where P(j) and U(j) denote parity and update indices in the tree, reducing the range of correlations compared to Jordan-Wigner while maintaining exact equivalence. Both transformations ensure the mapped Hamiltonian commutes with the total particle number and spin symmetries when appropriately tapered. Following the mapping, the second-quantized Hamiltonian decomposes into a sum of Pauli strings, the native basis for qubit operators: \hat{H} = \sum_k c_k \hat{P}_k, where each \hat{P}_k is a tensor product of single-qubit Pauli operators across the N qubits, and c_k are real coefficients derived from the integrals h_{pq} and h_{pqrs}. This Pauli encoding facilitates the VQE workflow by allowing the expectation value \langle \hat{H} \rangle to be computed variationally, though the number of terms can grow as O(N^4) for the two-electron part before sparsity exploitation. Jordan-Wigner tends to produce denser expansions with more high-weight terms, exacerbating circuit depth and error accumulation, whereas Bravyi-Kitaev yields sparser, lower-weight decompositions that better suit near-term hardware with limited connectivity. A key challenge in these encodings is the qubit overhead for realistic molecules: for example, simulating heavy elements like iron in biomolecules requires basis sets with hundreds of spin-orbitals, demanding correspondingly many qubits and exceeding current noisy intermediate-scale quantum devices limited to tens of qubits. Additionally, the choice between sparse (e.g., Bravyi-Kitaev, with fewer long-range terms) and denser (e.g., Jordan-Wigner) encodings trades off implementation simplicity against gate efficiency and noise resilience, with sparse variants reducing the overall resource demands but complicating circuit compilation on specific architectures. These mappings thus form the foundational step in preparing chemically relevant problems for VQE, directly influencing algorithmic scalability.

Algorithm Components

Ansatz Design

In the variational quantum eigensolver (VQE) algorithm, the serves as a parameterized that generates a trial wavefunction to approximate the of a target . This trial state is expressed as |\psi(\boldsymbol{\theta})\rangle = U(\boldsymbol{\theta}) |0\rangle, where U(\boldsymbol{\theta}) is a depending on variational parameters \boldsymbol{\theta}, and |0\rangle is typically an initial reference state such as the all-zero computational basis state. The 's role is to provide a flexible, ansatz-dependent manifold of states over which the minimizes the energy expectation value, enabling the identification of low-energy eigenstates on noisy intermediate-scale quantum devices. Ansatzes are broadly classified into hardware-efficient and problem-inspired types, each tailored to balance computational feasibility and representational power. Hardware-efficient ansatzes prioritize compatibility with current quantum hardware by employing shallow circuits composed of alternating layers of single-qubit rotation gates (e.g., R_x(\theta_i) and R_z(\theta_i)) and native entangling two-qubit gates (e.g., CNOT or ), often arranged in a pattern to minimize gate depth and mitigate noise. This design has demonstrated effectiveness in simulating small molecular Hamiltonians, such as \ce{H2} and \ce{LiH}, achieving chemical accuracy with reduced circuit overhead on superconducting qubit platforms. In contrast, problem-inspired ansatzes incorporate domain-specific , such as the unitary coupled-cluster singles and doubles (UCCSD) form, which emulates classical coupled-cluster theory by exponentiating anti-Hermitian operators corresponding to fermionic single and double excitations mapped to Pauli strings via Jordan-Wigner or Bravyi-Kitaev transformations. The UCCSD ansatz, U(\boldsymbol{\theta}) = e^{T(\boldsymbol{\theta}) - T^\dagger(\boldsymbol{\theta})}, where T includes excitation amplitudes, excels in applications by capturing effects with . Initial trial functions often begin with a physically motivated reference state to accelerate convergence and improve accuracy. In contexts, the Hartree-Fock () state—representing a mean-field approximation of the configuration—is commonly used as the starting point, prepared by applying a sequence of gates to encode the occupied orbitals into the register. Adaptive es, such as the adaptive derivative-assembled pseudo-Trotter (ADAPT) VQE, extend this by incrementally constructing the circuit: operators are selected from a predefined pool (e.g., fermionic excitations) based on their gradient magnitude with respect to the energy, building a compact layer-by-layer to enhance efficiency and reduce depth for molecules like \ce{LiH}. This approach has shown reductions to fewer than 50% of the parameters of fixed UCCSD forms while maintaining chemical accuracy. Key considerations in ansatz design revolve around the trade-off between expressivity—the ansatz's capacity to span a diverse set of quantum states approaching the true —and trainability, which ensures reliable optimization without encountering barren plateaus where gradients vanish exponentially. Highly expressive es, such as deep hardware-efficient circuits, risk trainability issues due to concentration of the energy landscape around its mean, leading to exponentially small gradients as system size increases; this phenomenon, analyzed in two-layer circuits, underscores the need for shallower, structured designs. To mitigate barren plateaus, practitioners favor es with limited depth (e.g., 1-2 layers) or symmetry-preserving elements, ensuring the variational landscape remains navigable for problems up to 20 qubits.

Measurement Protocol

In the variational quantum eigensolver (VQE), the protocol involves estimating the value of the encoded H = \sum_k c_k P_k, where c_k are coefficients and P_k are Pauli strings, to evaluate the energy of a trial state |\psi\rangle. This is achieved by computing \langle H \rangle = \sum_k c_k \langle P_k \rangle, with each \langle P_k \rangle obtained through projective on the quantum . For a given Pauli string P_k, the measurement basis is rotated via single-qubit gates to align with the eigenbasis of P_k, after which the circuit is executed multiple times () to sample measurement outcomes; the value is then estimated from the of +1 and -1 eigenvalues. To mitigate the high circuit depth and measurement overhead associated with measuring each P_k separately, Pauli terms are grouped into sets of mutually commuting operators, allowing simultaneous estimation in a single measurement basis per group. This reduces the number of required quantum circuits from the total number of Pauli terms (often scaling exponentially with system size) to the number of such commuting groups, which can be found using algorithms on the commutation graph of the terms. A prominent example is tapered measurements, which exploit Abelian symmetries (e.g., particle number or conservation) in the to eliminate redundant qubits and Pauli terms while preserving the spectrum, further lowering the measurement cost. For instance, in fermionic systems encoded via Jordan-Wigner or Bravyi-Kitaev transformations, up to $2^s terms can be tapered off, where s is the number of independent symmetries. Measurement errors arise primarily from shot noise, which introduces statistical variance inversely proportional to the number of shots per term, and readout errors, where misclassification of qubit states biases the estimates. These can be mitigated using zero-noise extrapolation (ZNE), which amplifies noise artificially (e.g., by inserting idle gates or ) and extrapolates the to the zero-noise limit via polynomial fitting, improving accuracy without additional hardware assumptions. Symmetry verification techniques complement this by post-selecting on measurement outcomes that respect the system's symmetries, discarding erroneous data and reducing bias from decoherence. The overhead remains a bottleneck, as the number of circuits scales linearly with the number of Pauli groups (typically O(N^4) for N-orbital Hamiltonians before grouping), requiring thousands to millions of for precision. Optimizations like quantum stochastic drift (qDRIFT) address this by probabilistically sampling Pauli terms with probabilities proportional to |c_k|, effectively estimating \langle H \rangle with fewer circuits at the cost of increased shot variance, which scales favorably for sparse or weakly correlated terms. This sampling approach can reduce the effective measurement cost by factors of 10–100 in practice for molecular simulations.

Classical Optimization

The classical optimization component of the variational quantum eigensolver (VQE) aims to minimize the variational energy expectation value E(\boldsymbol{\theta}) = \langle \psi(\boldsymbol{\theta}) | \hat{H} | \psi(\boldsymbol{\theta}) \rangle, where \boldsymbol{\theta} denotes the parameters of the quantum ansatz |\psi(\boldsymbol{\theta})\rangle = U(\boldsymbol{\theta}) |0\rangle and \hat{H} is the Hamiltonian. This minimization leverages the to approximate the ground-state energy, with the classical routine iteratively updating \boldsymbol{\theta} based on energy evaluations obtained from quantum measurements. The process integrates both gradient-based and algorithms, selected based on factors such as noise tolerance, computational cost, and the dimensionality of \boldsymbol{\theta}. For instance, gradient-based methods like , which employs adaptive moment estimates with hyperparameters such as learning rates and momentum coefficients, or L-BFGS, a quasi-Newton approach approximating the for efficient updates in low-dimensional spaces, require analytical gradients of E(\boldsymbol{\theta}). In contrast, derivative-free methods such as COBYLA, a by linear approximations algorithm that uses simplex-based searches, or Nelder-Mead, which performs direct landscape sampling without derivatives, are particularly robust in noisy quantum environments where gradient estimation may be unreliable. A for gradient-based optimization in VQE is the parameter-shift rule, which enables exact computation of partial derivatives \partial E / \partial \theta_k through additional evaluations. For Pauli rotation gates (e.g., R_x(\theta), R_y(\theta), R_z(\theta)) with standard generator coefficients, the rule computes the gradient as \frac{\partial \langle \hat{H} \rangle}{\partial \theta_k} = \frac{1}{2} \left[ \langle \hat{H} \rangle (\theta_k + s/2) - \langle \hat{H} \rangle (\theta_k - s/2) \right], where s = \pi is the shift parameter, requiring two shifted evaluations per parameter. This technique avoids errors and scales linearly with the number of parameters, though it doubles the quantum calls compared to energy evaluations alone; extensions to multi-parameter gates use stochastic sampling for efficiency. The hybrid quantum-classical loop orchestrates this by repeatedly invoking the quantum device as an to compute E(\boldsymbol{\theta}) or shifted expectations, followed by classical updates to \boldsymbol{\theta} until convergence. This iterative feedback, often implemented in frameworks like or PennyLane, ensures the evolves toward lower energies while mitigating quantum hardware limitations. Convergence is typically monitored through criteria such as an energy threshold (e.g., achieving chemical accuracy of 1.6 mHartree relative to the exact ) or a small (e.g., \|\nabla E(\boldsymbol{\theta})\| < 10^{-6}), halting the optimization when either is satisfied to balance accuracy and resource use. Local minima, a common challenge due to the non-convex energy landscape, are addressed via warm-starting techniques that initialize \boldsymbol{\theta} near promising regions using approximations from classical solvers, prior VQE runs on similar systems, or reduced ansatzes, thereby accelerating convergence and improving solution quality. For example, warm-starting with solutions from simpler molecular geometries has been shown to reduce iteration counts by providing better initial guesses, enhancing overall efficiency in practical VQE applications.

Mathematical Formulation

Core Equations

The variational quantum eigensolver (VQE) relies on minimizing a parameterized cost function to approximate the ground-state energy E_0 of a quantum Hamiltonian H. The core cost function is the expectation value of the Hamiltonian with respect to a parameterized trial wavefunction |\psi(\theta)\rangle, given by E(\theta) = \langle \psi(\theta) | H | \psi(\theta) \rangle, assuming the trial state is normalized such that \langle \psi(\theta) | \psi(\theta) \rangle = 1. In the more general unnormalized form introduced in the original formulation, it is the Rayleigh quotient E(\theta) = \frac{\langle \psi(\theta) | H | \psi(\theta) \rangle}{\langle \psi(\theta) | \psi(\theta) \rangle}, which is minimized over the variational parameters \theta to yield an upper bound on E_0. The expectation value \langle H \rangle can be expressed using the density operator \rho(\theta) = |\psi(\theta)\rangle \langle \psi(\theta) |, as \langle H \rangle = \mathrm{Tr} [\rho(\theta) H]. For practical computation on quantum hardware, the Hamiltonian is typically decomposed into a linear combination of Pauli operators: H = \sum_k c_k P_k, where c_k are real coefficients and P_k are tensor products of Pauli matrices. The expectation then becomes \langle H \rangle = \sum_k c_k \langle P_k \rangle, with each \langle P_k \rangle = \langle \psi(\theta) | P_k | \psi(\theta) \rangle obtained via quantum measurements. At the variational minimum, the condition \frac{\partial E}{\partial \theta_j} = 0 holds for each parameter \theta_j. Differentiating the cost function yields \frac{\partial E}{\partial \theta_j} = 2 \mathrm{Re} \left[ \left\langle \frac{\partial \psi(\theta)}{\partial \theta_j} \Big| H - E(\theta) \Big| \psi(\theta) \right\rangle \right] = 0, which leverages the Hellmann-Feynman theorem in the context of parameter-shift rules or finite-difference approximations for gradient evaluation during classical optimization. The variational principle guarantees convergence to the exact ground-state energy: E(\theta) \geq E_0 for any trial state, with equality achieved in the limit as the ansatz |\psi(\theta)\rangle spans the full Hilbert space of the system.

Algorithm Steps

The variational quantum eigensolver (VQE) operates through an iterative hybrid quantum-classical procedure to approximate the ground state energy of a given Hamiltonian. The steps are outlined below in a structured format, drawing from the original formulation and subsequent refinements for practical implementation.
  1. Encode the Hamiltonian into Pauli observables. The input Hamiltonian H, representing the quantum system of interest (e.g., from quantum chemistry or materials simulation), is transformed into a qubit-based representation. This involves mapping fermionic or other operators to a sum of Pauli strings: H = \sum_k c_k P_k, where c_k are coefficients and P_k are tensor products of Pauli matrices (I, X, Y, Z). Common mappings include the Jordan-Wigner or Bravyi-Kitaev transformations to ensure the encoding is compatible with qubit hardware. This step enables the expectation value \langle H \rangle to be computed additively from measurements of the individual P_k.
  2. Initialize ansatz parameters \theta. A parameterized quantum circuit, or ansatz, is selected to generate trial states within a variational manifold. The parameters \theta (e.g., rotation angles in the circuit) are initialized, often starting from a mean-field solution such as the to provide a physically motivated initial guess close to the ground state. Random initialization may also be used in some cases.
  3. Quantum evaluation: Prepare |\psi(\theta)\rangle and measure \langle H \rangle via Pauli grouping. The trial state |\psi(\theta)\rangle is prepared on a quantum processor by executing the ansatz circuit with the current \theta. The energy E(\theta) = \langle \psi(\theta) | H | \psi(\theta) \rangle is estimated by measuring the expectation values \langle P_k \rangle for each Pauli term, typically grouped into commuting sets to minimize the number of distinct quantum circuits required (e.g., via qubit-wise or full commutativity partitioning). Multiple shots are performed per group to reduce statistical error. Measurement techniques are detailed in the Measurement Protocol section.
  4. Classical update: Optimize \theta to minimize E(\theta); iterate until convergence. The estimated E(\theta) is passed to a classical computer, where an optimization routine (e.g., gradient-based or derivative-free methods) updates \theta to lower the energy. This quantum-classical feedback loop repeats, with the quantum evaluation providing the objective function evaluations for the optimizer.
Upon termination—typically when the change in E(\theta) falls below a predefined threshold or a maximum iteration count is reached—the algorithm outputs the minimized energy as an approximation to the ground state eigenvalue and the final |\psi(\theta)\rangle as the corresponding eigenvector, which can be reconstructed classically or via additional quantum measurements.

Implementations and Examples

Basic Example

A basic example of the variational quantum eigensolver (VQE) involves computing the ground state energy of the hydrogen molecule (H₂) at its equilibrium bond length of 0.74 Å. This system is modeled with the STO-3G minimal basis set, yielding 4 spin-orbitals to describe the 2 electrons. The second-quantized electronic Hamiltonian is mapped to a qubit operator via the Jordan-Wigner transformation, resulting in a minimal model comprising 4 Pauli terms. The variational ansatz employs the unitary coupled cluster singles and doubles (UCCSD) form, featuring 2 parameters corresponding to the single and double excitation amplitudes. This ansatz is prepared starting from the , which serves as the initial trial wavefunction. A classical optimizer, such as sequential least squares programming, iteratively adjusts the parameters to minimize the expectation value of the encoded Hamiltonian. Upon convergence, the VQE yields a ground state energy of approximately -1.136 Hartree, aligning closely with the full configuration interaction (FCI) benchmark for this system and demonstrating chemical accuracy within 1.6 mHartree. This example highlights VQE's ability to approximate molecular ground states using a compact ansatz and limited qubit resources.

Software Tools

Several open-source software libraries and frameworks have been developed to facilitate the implementation of the variational quantum eigensolver (VQE), enabling both simulations on classical hardware and execution on quantum devices. These tools typically provide modules for constructing quantum Hamiltonians, designing parameterized ansatze, performing measurements, and integrating classical optimization routines, often with support for noisy intermediate-scale quantum (NISQ) devices. Qiskit, developed by IBM, includes comprehensive support for VQE through its Qiskit Nature module (formerly part of Qiskit Aqua), which offers pre-built ansatze such as the unitary coupled-cluster (UCC) singles and doubles (UCCSD) for quantum chemistry applications. This framework allows users to simulate VQE workflows on classical backends or execute them on IBM's cloud-accessible quantum hardware, with built-in error mitigation techniques like zero-noise extrapolation. Qiskit's integration with the Optimization module further enables the use of classical solvers such as COBYLA or SPSA for minimizing the variational energy. Cirq, Google's quantum computing framework, provides VQE implementations through its experiments and contrib packages, including tutorials for variational algorithms, supporting the creation of custom circuits and expectation value computations for molecular Hamiltonians. It integrates seamlessly with for automatic differentiation, allowing efficient computation of parameter gradients essential for gradient-based optimization in VQE. Cirq's design emphasizes flexibility for NISQ devices, including support for Google's quantum processors through the Cirq Google extension. PennyLane, from Xanadu, specializes in differentiable quantum programming and supports hybrid quantum-classical VQE implementations through its quantum machine learning primitives. Users can define VQE circuits with hardware-agnostic ansatze and leverage built-in optimizers like Adam or Rotosolve, with automatic differentiation for both quantum and classical components. Notably, PennyLane extends VQE to photonic quantum hardware via plugins for platforms like Strawberry Fields, enabling simulations of continuous-variable systems alongside discrete qubit-based approaches. OpenFermion, an open-source library focused on quantum simulations of fermionic systems, provides essential tools for VQE by facilitating the construction of second-quantized Hamiltonians from molecular integrals and generating fermionic ansatze like Jordan-Wigner or Bravyi-Kitaev transformations. It serves as a foundational layer that integrates with higher-level frameworks such as or for full VQE pipelines, emphasizing accurate mapping of quantum chemistry problems to qubit operators without direct hardware execution.

Applications

Quantum Chemistry

The variational quantum eigensolver (VQE) plays a pivotal role in quantum chemistry by enabling the simulation of molecular electronic structures through the approximation of ground-state wavefunctions and energies. By optimizing a parameterized quantum circuit to minimize the expectation value of the molecular —encoded into qubit operators via fermion-to-qubit mappings such as the —VQE facilitates accurate predictions for systems intractable on classical computers. Early applications focused on small molecules, demonstrating VQE's potential to rival high-level ab initio methods. For ground-state energies, VQE using the unitary coupled-cluster singles and doubles (UCCSD) in the STO-3G basis has computed values for LiH and BeH2 within chemical accuracy (1.6 mHa) of full interaction (FCI) benchmarks, requiring 12 qubits for LiH and 14 for BeH2. These results highlight VQE's efficacy for molecules with up to 6 electrons, where the UCCSD captures strong effects effectively. curves for LiH, generated by varying lengths from 0.7 to 10 Å, show VQE/UCCSD profiles with errors below 0.07 Ha relative to FCI, closely reproducing the and behavior observed in classical computations. Similar accuracy is achieved for BeH2 linear configurations, underscoring VQE's utility in mapping surfaces for reactive processes. Extensions of VQE, such as adaptive VQE-X, target excited states by iteratively building ansätze that minimize variance while ensuring to lower eigenstates, extending the ground-state framework to higher-energy spectra. For LiH in the STO-3G basis, VQE-X variants compute the first and triplet excited states with chemical accuracy against FCI using 12 qubits, enabling the study of photochemical transitions. Reaction , crucial for understanding chemical reactivity, have been estimated via VQE; for example, the of cyclohexadiene (C6H8 + H2) yields barriers and exothermicity in semi-quantitative agreement with FCI, differing by less than 0.01 at key geometries. To address larger systems, VQE integrates with classical embedding techniques, such as , which partitions molecules into a quantum-active subspace and a classically treated environment, reducing qubit demands. Embedded VQE applied to C6H8 + H2 achieves coupled-cluster singles and doubles (CCSD) accuracy using 16 qubits, compared to 68 for the full system, while correctly predicting equilibrium geometries for polyynes like C18 with 16 qubits versus 144. A 2024 advance, fragment molecular orbital-based VQE (FMO-VQE), further enhances scalability by fragmenting molecules and applying VQE to monomer and dimer interactions; for neutral hydrogen clusters like H6 and anionic H5- in the 6-31G basis, it delivers ground-state energies and reaction energies with errors below 0.2 mHa relative to CCSD, using at most 8 . Benchmarks indicate VQE matches CCSD(T) accuracy for small molecules (e.g., LiH errors <1 mHa), but scales less favorably for larger systems without hybridization. For molecules with more than 10 orbitals, such as C2H4 (14 spatial orbitals in STO-3G), 28–32 qubits are typically required for chemical accuracy versus FCI, though reduces this to 10–16 qubits while maintaining CCSD-level precision. These integrations position VQE as a hybrid tool for realistic simulations beyond current classical limits.

Other Domains

The variational quantum eigensolver (VQE) has found significant applications in , particularly for modeling spin systems described by Heisenberg and Ising Hamiltonians. In studies of antiferromagnetic Heisenberg models on frustrated lattices like the structure, VQE has been employed to approximate ground states, revealing insights into highly degenerate energy landscapes and magnetic ordering. For instance, simulations on quantum hardware have demonstrated VQE's ability to prepare states for small lattices, achieving energies close to classical benchmarks despite noise. Similarly, the has been simulated using VQE to probe quantum phase transitions, such as those induced by boundary conditions or in two-dimensional systems. Recent 2025 experiments on superconducting qubits have shown VQE capturing phase boundaries with chemical accuracy for chains up to 10 spins, highlighting its utility in studying glassy dynamics and ordered phases. In optimization problems, VQE has been integrated with the quantum approximate optimization algorithm (QAOA) in hybrid frameworks to tackle combinatorial challenges. These hybrids encode problems like or traveling salesperson instances into Ising-like Hamiltonians, where VQE optimizes variational parameters to minimize objective functions. A 2025 study applied such a QAOA-VQE approach to instances, outperforming classical heuristics in ratios for moderately sized graphs on noisy intermediate-scale quantum devices. Additionally, VQE facilitates solving partial equations (PDEs) by discretizing them into Hamiltonians, as demonstrated in 2025 work on the advection-diffusion equation. Here, VQE on a finite-difference approximates ground-state solutions, yielding velocity fields with errors below 5% for low Reynolds numbers, offering a quantum advantage in high-dimensional simulations. Within , VQE has advanced the computation of electronic properties in periodic systems, including band structures and defect energies. For band structures in , a 2025 hybrid quantum-classical method combined VQE with quantum subspace expansion to calculate dispersion relations in Hubbard models, achieving convergence to within 1 meV of results for small supercells. Tailored ansatze for multi-band tight-binding Hamiltonians have enabled VQE to determine band gaps in metal-halide perovskites, with 2025 simulations on 20- circuits providing accurate predictions for finite-sized systems relevant to . Regarding defects, VQE has been used to evaluate spin defect energies in solid-state hosts, such as nitrogen-vacancy centers in ; a 2025 ADAPT-VQE implementation reduced qubit overhead while estimating formation energies to chemical precision, aiding quantum sensing applications. In high-energy physics, VQE approximations have been explored for lattice (QCD), focusing on Yang-Mills vacua and gauge theories. Early applications targeted SU(3) plaquette chains, where VQE prepared low-energy states with exceeding 90% on small lattices. More recent 2025 efforts incorporated irreducible representations and to mitigate barren plateaus, enabling VQE to approximate ground states of lattice QCD Hamiltonians for volumes up to 2x2x2, with applications to and confinement properties.

Advantages and Challenges

Benefits

The variational quantum eigensolver (VQE) is particularly well-suited for noisy intermediate-scale quantum (NISQ) devices due to its reliance on shallow quantum circuits that require shorter coherence times and exhibit greater tolerance to noise compared to algorithms like quantum phase estimation, thereby eliminating the immediate need for full . This design allows VQE to leverage current quantum hardware with limited counts, typically in the range of tens to hundreds of qubits, while maintaining computational viability in the presence of imperfect gates and decoherence. A key strength of VQE lies in its hybrid quantum-classical architecture, which offloads the computationally intensive optimization process—such as parameter updates via classical routines like —to a conventional computer, while the quantum handles and evaluation. This division not only reduces the burden on the quantum hardware but also enables iterative refinement of trial wavefunctions through repeated short quantum measurements, trading extended quantum coherence for a increase in classical processing overhead. VQE offers substantial flexibility through its use of parameterized circuits, which can be tailored to specific problem domains using chemically inspired forms like unitary coupled cluster or hardware-efficient constructions, allowing adaptation to both the molecular system and the underlying quantum architecture. Beyond ground-state energies, the approach facilitates additional insights such as state by estimating reduced matrices or excited states via extensions like quantum subspace methods, providing a versatile framework for analysis. Regarding scalability, VQE holds promise for achieving chemical accuracy—defined as energies within 1.6 mHa of the exact value—for systems requiring more than 50 qubits when combined with error mitigation techniques such as zero-noise extrapolation or probabilistic error cancellation, which correct for noise with modest additional measurement costs. As of 2025, demonstrations have extended to systems requiring up to 50 qubits using advanced variants like FAST-VQE. This potential stems from the variational principle's guarantee of an upper bound on the energy, enabling progressive improvements as hardware advances.

Limitations

The variational quantum eigensolver (VQE) is highly sensitive to inherent in current noisy intermediate-scale quantum (NISQ) devices, where decoherence and gate errors degrade the accuracy of expectation value measurements. To achieve reliable estimates amid statistical fluctuations and systematic biases from imperfect operations, VQE typically requires more than 10^3 measurement shots per Pauli term in the , with final energy evaluations often demanding up to 10^5 shots to approach chemical accuracy of 1.6 mHa. This overhead arises because decoherence shortens depths to mere 0–2 layers for optimal performance, limiting the expressivity of trial states and amplifying errors in larger systems. A major trainability challenge in VQE stems from barren plateaus, where the variance of gradients in the vanishes exponentially with the number of qubits N, scaling as O(2^{-N}) for random parameter initializations in expressive ansätze. This phenomenon, prevalent in deep parameterized quantum circuits, makes classical optimization inefficient as parameter updates become vanishingly small, often below chemical precision thresholds. While mitigations like careful initialization strategies can alleviate this issue for shallow circuits, it remains a fundamental barrier for scaling to problem sizes beyond tens of qubits. Resource demands in VQE scale unfavorably for quantum chemistry applications, with the second-quantized molecular Hamiltonian decomposing into O(N^4) Pauli terms under the Jordan-Wigner mapping, where N is the number of spin orbitals. This results in a measurement overhead linear in the number of terms, requiring O(N^4 / \epsilon^2) total shots per optimization iteration for precision \epsilon, though grouping techniques can reduce it to O(N^3). Circuit depths and gate counts further escalate with ansatz complexity, such as O(N^4) two-qubit gates for unitary coupled-cluster ansätze, constraining practical implementations to small molecules like H_2 or LiH on current hardware. VQE's optimization landscape is non-convex and prone to local minima, heavily dependent on the choice of , which may not span the full and thus yields only an upper bound to the true ground-state energy per the . Incomplete or poorly expressive , such as hardware-efficient variants, can trap the algorithm in suboptimal solutions, with rates deteriorating exponentially in system size due to narrow gorges in the energy landscape. This ansatz reliance underscores the need for problem-tailored trial states, yet no choice guarantees optimality.

Recent Developments

Variants and Improvements

Since its inception, the variational quantum eigensolver (VQE) has seen significant enhancements through adaptive constructions that dynamically build parameterized quantum circuits tailored to the problem at hand. The adaptive derivative-assembled pseudo-Trotter (ADAPT)-VQE algorithm, introduced in 2019, iteratively selects operators based on their gradient magnitudes to construct a compact , reducing circuit depth while improving convergence for molecular ground states. Extensions in 2023 have refined ADAPT-VQE by incorporating problem-tailored operator pools that account for local electronic structure, enhancing accuracy on noisy intermediate-scale quantum (NISQ) hardware for systems like the hydrogen molecule. Another 2023 variant, Overlap-ADAPT-VQE, leverages overlap measurements between trial states and reference configurations to further optimize selection, demonstrating reduced parameter counts and better scalability for simulations. To address optimization challenges such as barren plateaus—regions in the parameter landscape where gradients vanish, hindering training—a cyclic VQE framework was proposed in 2025. This approach employs a hardware-efficient with measurement-driven feedback loops that enable "staircase descent," allowing escape from plateaus by cyclically adjusting parameters in a structured manner, achieving ground-state energies within 1% chemical accuracy for up to 20-qubit systems on simulated NISQ devices. Error mitigation techniques have been integrated into VQE workflows to counteract noise in NISQ environments without requiring full error correction. QDRIFT, a randomized simulation method that averages noisy circuit outcomes to approximate ideal expectations, has been applied to VQE for ground-state in noisy simulations. Complementing this, probabilistic error cancellation (PEC) inverts the noise channel by sampling quasi-probability distributions of gate sequences, yielding unbiased estimates; when combined with VQE, PEC has mitigated errors in various platforms, with feasible sampling overheads. A 2025 distributed VQE variant extends these mitigations across networked quantum processors for (QUBO) problems, partitioning for parallel computation while synchronizing via classical links. Specialized VQE adaptations target non-standard quantum states and optimization paradigms. The variational quantum state eigensolver (VQSE), developed in 2022, extends VQE to mixed states by variationally optimizing the largest eigenvalues of density matrices, preparing corresponding eigenstates via a parameterized ; this has proven effective for state simulations in open quantum systems, such as chains at finite temperatures. Building on adaptive principles, a greedy gradient-free adaptive VQE (GGA-VQE) was introduced in 2025, which selects operators via analytic, derivative-free metrics like energy gradients, avoiding costly quantum gradient computations; tested on a 25-qubit trapped-ion for Ising models, it converged to ground states 2-3 times faster than standard parameter-shift methods while maintaining depths under 100 gates. Efficiency improvements for large-scale applications have focused on fragmentation strategies. The fragment molecular orbital (FMO)-based VQE, proposed in 2024, divides macromolecules into interacting fragments, solving reduced Hamiltonians per fragment with VQE before perturbatively reconstructing the full ; demonstrated on small systems like the dimer, this approach efficiently utilizes qubits for simulations. As of November 2025, recent advances include full simulations of 50-qubit quantum computers for VQE , parallelized Givens ansatzes for molecular states, and stabilizer-accelerated methods for many-body , enhancing on NISQ hardware.

Experimental Realizations

One of the earliest experimental realizations of the variational quantum eigensolver (VQE) was demonstrated using trapped-ion qubits in 2018, where researchers implemented a scalable version to compute the ground-state energies of the H₂ and LiH molecules. This experiment, conducted on a digital quantum simulator with four qubits, achieved energies within 0.4% of the full configuration interaction values, marking the first hardware demonstration of VQE for quantum chemistry problems despite noise limitations. In parallel, superconducting platforms advanced VQE implementations starting in , with experiments on IBM's early quantum processors optimizing up to six- Hamiltonians derived from molecular structures like H₂ and LiH in minimal bases. These hardware-efficient ansatze, tailored to reduce depth, yielded ground-state energies with errors below % relative to exact , highlighting VQE's resilience to gate fidelities around 99%. A related demonstration involved preparing a five- GHZ state as part of benchmarking VQE's performance on correlated systems. Mid-scale experiments expanded to larger systems by 2019, exemplified by VQE runs on IBM's 20-qubit superconducting processor for simulating hydrides such as LiH. Using a unitary coupled-cluster , these tests benchmarked VQE against classical methods, achieving chemical accuracy (error < 1.6 mHa) for small molecules after error mitigation, though circuit depths up to 100 gates posed challenges for NISQ . Photonic platforms contributed to VQE realizations around 2021, particularly for bosonic systems, with continuous-variable implementations on Xanadu's encoding the of the attractive Bose-Hubbard model for up to four modes. This approach leveraged Gaussian states and non-Gaussian operations to capture strong correlations, demonstrating fidelity improvements over mean-field approximations in noisy photonic setups. Recent advancements by 2023 focused on scaling beyond 50 qubits with error mitigation techniques, as shown in trapped-ion experiments using purification methods to enhance VQE accuracy for pair-correlated models. On IonQ's 32-qubit , these runs mitigated readout and gate errors, reducing estimation variance by factors of 10–100, enabling feasible approximations for systems requiring 50+ qubits without full . Distributed VQE architectures have been explored in theoretical proposals as of 2024, including partitioning circuits across modules connected via limited entanglement links for scalability in multi-node setups. Benchmarks in 2024 underscored VQE's progress toward chemical accuracy on real hardware, with photonic qudit-based experiments estimating LiH ground-state energies to within 0.036 Ha of full configuration interaction results using orbital-angular-momentum encoding on four qudits. Error rates around 5% were reported, with fidelities exceeding 90% for key gates, establishing VQE's viability for small-molecule quantum chemistry under NISQ constraints.

References

  1. [1]
    A variational eigenvalue solver on a photonic quantum processor
    Jul 23, 2014 · ... Peruzzo et al. develop a variational computation ... Gate-free state preparation for fast variational quantum eigensolver simulations.
  2. [2]
  3. [3]
  4. [4]
    Hardware-efficient variational quantum eigensolver for ... - Nature
    Sep 14, 2017 · Here we demonstrate the experimental optimization of Hamiltonian problems with up to six qubits and more than one hundred Pauli terms, ...
  5. [5]
    [1808.10402] Quantum computational chemistry - arXiv
    Aug 30, 2018 · This review provides a comprehensive introduction to both computational chemistry and quantum computing, bridging the current knowledge gap.
  6. [6]
    None
    ### Summary of Variational Principle and Related Sections from arXiv:1304.3061
  7. [7]
    [PDF] Theory of variational quantum simulation - arXiv
    In this work, we first review the conventional variational principles, including the Rayleigh-Ritz method for solving static problems, and the Dirac and Frenkel ...
  8. [8]
    [PDF] On the Rayleigh-Ritz variational method - arXiv
    Nov 5, 2023 · We give a simple proof of the well known fact that the approximate eigenvalues provided by the Rayleigh-Ritz variational method are increas-.
  9. [9]
    The Variational Quantum Eigensolver: a review of methods and best ...
    Nov 9, 2021 · The variational quantum eigensolver (or VQE) uses the variational principle to compute the ground state energy of a Hamiltonian.Missing: primary | Show results with:primary
  10. [10]
    Simulated Quantum Computation of Molecular Energies - Science
    Sep 9, 2005 · These simulations show that quantum computers of tens to hundreds of qubits can match and exceed the capabilities of classical FCI calculations.
  11. [11]
    [quant-ph/0003137] Fermionic quantum computation - arXiv
    Mar 29, 2000 · We define a model of quantum computation with local fermionic modes (LFMs) -- sites which can be either empty or occupied by a fermion.Missing: original | Show results with:original
  12. [12]
    VQE method: a short survey and recent developments
    Jan 6, 2022 · The variational quantum eigensolver (VQE) is a method that uses a hybrid quantum-classical computational approach to find eigenvalues of a Hamiltonian.Introduction To Vqe · Hardware-Efficient Ansatzes · Qubit Coupled Cluster Method
  13. [13]
    [1704.05018] Hardware-efficient Variational Quantum Eigensolver ...
    Apr 17, 2017 · Hardware-efficient Variational Quantum Eigensolver for Small Molecules and Quantum Magnets. Authors:Abhinav Kandala, Antonio Mezzacapo, Kristan ...
  14. [14]
    Qubit coupled cluster singles and doubles variational quantum ...
    May 18, 2020 · Among all proposed VQE algorithms, the unitary coupled cluster singles and doubles excitations (UCCSD) VQE ansatz has achieved high accuracy and ...
  15. [15]
    An adaptive variational algorithm for exact molecular simulations on ...
    Jul 8, 2019 · ... VQE approach for systems which are not well described with unitary coupled cluster. In order to perform the simulations, an in-house code ...
  16. [16]
    Connecting Ansatz Expressibility to Gradient Magnitudes and ...
    Jan 24, 2022 · Our results do not preclude inexpressive ansatze having trainability issues, such as barren plateaus. On the other hand, highly expressive ...Missing: VQE | Show results with:VQE
  17. [17]
    [2312.08105] Towards determining the presence of barren plateaus ...
    Dec 13, 2023 · Our results emphasize the link between trainability and circuit expressiveness, raising doubts about VQEs' ability to surpass classical methods.
  18. [18]
    [1701.08213] Tapering off qubits to simulate fermionic Hamiltonians
    Jan 27, 2017 · The paper discusses encoding fermionic systems with qubits, eliminating redundant degrees of freedom to enable quantum simulations with fewer  ...
  19. [19]
    Evaluating analytic gradients on quantum hardware | Phys. Rev. A
    Mar 21, 2019 · In many cases of qubit-based quantum computing the derivatives can be computed with a simple parameter shift rule, using the variational ...
  20. [20]
    [2107.12390] General parameter-shift rules for quantum gradients
    Jul 26, 2021 · In this work, we use this fact to derive new, general parameter-shift rules for single-parameter gates, and provide closed-form expressions to apply them.Missing: original | Show results with:original
  21. [21]
    Accelerating variational quantum eigensolver convergence using ...
    Aug 4, 2023 · In this work, we evaluate a quantum computational warm-start approach for potential energy surface calculations.
  22. [22]
  23. [23]
    The theory of variational hybrid quantum-classical algorithms - arXiv
    Sep 14, 2015 · A quantum-classical hybrid optimization scheme known as the quantum variational eigensolver was developed with the philosophy that even minimal quantum ...
  24. [24]
    [PDF] Simulating molecules using the VQE algorithm on Qiskit - arXiv
    Jan 8, 2022 · For this particular case, we chose to employ the Unitary Couple Cluster (UCCSD) as our variational form and the Sequential Least Squares ...
  25. [25]
    Frontiers | Benchmarking Adaptive Variational Quantum Eigensolvers
    **Summary of H₂ Molecule Details in STO-3G Basis Using VQE with UCCSD Ansatz:**
  26. [26]
    [PDF] Benchmarking the Variational Quantum Eigensolver using different ...
    May 11, 2023 · In the particular study within this paper, we concentrate on simulating the H2 molecule as a basic use case for comparing superconducting and ...
  27. [27]
    Converting the result of expval Hamilton to eV - PennyLane Help
    Apr 12, 2024 · ... STO-3G") h2 = h2_dataset[0] H ... The ground state energy for an H2 molecule is about -31eV which indeed corresponds to -1.136 Hartree.
  28. [28]
    Barren plateaus in quantum neural network training landscapes
    Nov 16, 2018 · McClean, J. R., Romero, J., Babbush, R. & Aspuru-Guzik, A. The theory of variational hybrid quantum-classical algorithms. New J. Phys. 18 ...
  29. [29]
  30. [30]
    Adaptive, problem-tailored variational quantum eigensolver ... - Nature
    Mar 1, 2023 · In this work, we consider the Adaptive, Problem-Tailored Variational Quantum Eiegensolver (ADAPT-VQE) ansätze, and examine how they are impacted by these local ...<|separator|>
  31. [31]
    Overlap-ADAPT-VQE: practical quantum chemistry on ... - Nature
    Jul 29, 2023 · ADAPT-VQE is a robust algorithm for hybrid quantum-classical simulations of quantum chemical systems on near-term quantum computers.
  32. [32]
    Cyclic Variational Quantum Eigensolver: Escaping Barren Plateaus ...
    Sep 16, 2025 · We introduce the Cyclic Variational Quantum Eigensolver (CVQE), a hardware-efficient framework for accurate ground-state quantum simulation on ...
  33. [33]
    Error mitigation in variational quantum eigensolvers using tailored ...
    Jul 15, 2024 · In this paper, we present a method that employs parametric Gaussian process regression (GPR) within an active learning framework to mitigate noise in quantum ...
  34. [34]
    Distributed Implementation of Variational Quantum Eigensolver to ...
    Aug 24, 2025 · This near-optimal initialization is a warm start for the VQE training loop, reducing iterations and improving convergence.
  35. [35]
    Variational quantum state eigensolver | npj Quantum Information
    Sep 21, 2022 · We introduce the variational quantum state eigensolver (VQSE), which is analogous to VQE in that it variationally learns the largest eigenvalues of ρ as well ...
  36. [36]
    Greedy gradient-free adaptive variational quantum algorithms on a ...
    May 28, 2025 · We introduce an adaptive algorithm using analytic, gradient-free optimization, called Greedy Gradient-free Adaptive VQE (GGA-VQE).Missing: qDRIFT | Show results with:qDRIFT
  37. [37]
    Fragment molecular orbital-based variational quantum eigensolver ...
    Jan 29, 2024 · The primary objective of the VQE is to minimize the expectation value of the Hamiltonian for a given trial wave function by finding the optimal ...<|control11|><|separator|>
  38. [38]
    Quantum Chemistry Calculations on a Trapped-Ion Quantum ...
    Jul 24, 2018 · We report on the experimental implementation of such an algorithm to solve a quantum chemistry problem, using a digital quantum simulator based on trapped ions.Missing: H2 | Show results with:H2
  39. [39]
    Quantum chemistry as a benchmark for near-term quantum computers
    Nov 15, 2019 · Kandala, A. et al. Hardware-efficient variational quantum eigensolver for small molecules and quantum magnets. Nature 549, 242–246 (2017).
  40. [40]
    Encoding strongly-correlated many-boson wavefunctions on a ...
    Nov 8, 2021 · In this work, we investigate the encoding of the ground state of the (simple but rich) attractive Bose-Hubbard model using a Continuous-Variable (CV) photonic- ...
  41. [41]
    Purification-based quantum error mitigation of pair-correlated ...
    Oct 12, 2023 · For instance, successfully implementing a 50-qubit VQE with ansatz depth 3N2/2 with EV or VD would require error rates to drop ~1,000×.
  42. [42]
    Distributed quantum computing: A survey - ScienceDirect.com
    IBM plans to introduce in 2025 Kookaburra – a 1386 qubit multi-chip processor with communication link support for quantum parallelization – with three ...
  43. [43]
    Qudit-based variational quantum eigensolver using photonic orbital ...
    Oct 23, 2024 · In this work, we experimentally demonstrate a single qudit–based variational quantum eigensolver (SQD-VQE) using OAM states of a single photon.